Size-dependent picosecond energy relaxation in PbSe quantum dots
نویسندگان
چکیده
منابع مشابه
Excited-state relaxation in PbSe quantum dots.
In solids the phonon-assisted, nonradiative decay from high-energy electronic excited states to low-energy electronic excited states is picosecond fast. It was hoped that electron and hole relaxation could be slowed down in quantum dots, due to the unavailability of phonons energy matched to the large energy-level spacings ("phonon-bottleneck"). However, excited-state relaxation was observed to...
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Triplet-singlet spin relaxation in a vertical electrostatic quantum dot containing two interacting electrons is studied with a realistic model that includes the effects of finite thickness and screening. The spin relaxation mechanism is taken to be spin mixing via the part of the Dresselhaus Hamiltonian that is linear in the lateral momentum. The electron-electron interaction enhances relaxatio...
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We investigated the effect of PbSe quantum dot size on the performance of Schottky solar cells made in an ITO/PEDOT/PbSe/aluminum structure, varying the PbSe nanoparticle diameter from 1 to 3 nm. In this highly confined regime, we find that the larger particle bandgap can lead to higher open-circuit voltages (∼0.6 V), and thus an increase in overall efficiency compared to previously reported de...
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Different sizes of three-dimensional PbSe quantum dots have been synthesized for the study of orbital magnetic susceptibilities. Two types of orbital susceptibilities have been found, including the Curie susceptibility and finite-size corrections to the Landau susceptibility. The Curie term of a quantum dot manifests itself in the temperature dependence of magnetic susceptibility at low tempera...
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The spectroscopic behavior of colloidal InP quantum dots (QDs) has been investigated as a function of the mean QD diameter (which ranged from 26 to 60 Å). Absorption spectra show up to three peaks or shoulders which reflect excited state transitions in the QDs. Global photoluminescence (PL) spectra (excitation well to the blue of the absorption onset and which consequently excites most of the Q...
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ژورنال
عنوان ژورنال: Applied Physics Letters
سال: 2000
ISSN: 0003-6951,1077-3118
DOI: 10.1063/1.127025